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We study the decay kinetics of excited state of GR1 center in diamond using 633 nm pump pulse and 658 nm CW probe beam. The absorption saturation followed by a strong absorption of the probe below steady-state transmission level was observed. The recovery of the centers to the original level occurs slowly with ~500 ns time scale and reveals multi-exponential rates with no long-term bleaching or residual absorption. The branching ratio for relaxation process to the ground state and to the metastable state was estimated to be ~ 0.50.
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Shova D. Subedi, Vladimir V. Fedorov, Sergey Mirov, Matthew Markham, "Study of relaxation dynamics of excited state of GR1 centers in diamond," Proc. SPIE 11664, Solid State Lasers XXX: Technology and Devices, 116640K (5 March 2021); https://doi.org/10.1117/12.2583168