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Modulating the electronic, magnetic and optical properties at the molecular level using an external trigger has been
extended to the field of nonlinear optics. The switching molecule is designed to have a complexation site or a redox
active unit which can guarantee electronic communication over the whole conjugated system. The alteration of the
nonlinear property is then induced by the modulation of the internal charge-transfer due to the response of the molecule
to the external stimulus. This can be achieved by cation binding, protonation/deprotonation or electrochemically.
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Inge Asselberghs, Gunther Hennrich, Benjamin J. Coe, Koen Clays, "Control and switching of first hyperpolarizability by pH," Proc. SPIE 6331, Linear and Nonlinear Optics of Organic Materials VI, 633104 (14 September 2006); https://doi.org/10.1117/12.678027