Through the combination of nanoscale Mie-resonance and photothermal/thermo-optical effect, the nonlinear index n2 of both plasmonic and metal nanostructure can be enhanced by more than three orders of magnitude. We discovered various types of nonlinearity that include saturation, suppression, and reverse saturation in nanostructures. Through a similar mechanism, we also achieved optical bistability in a nanoscale resonator with a record-low Q-factor (<10) and observed large nonlinearity with hysteretic behavior. These tunable optical nonlinearities with low requirements on sample size and shape open new possibilities for the design of photonic devices and metal/semiconductor super-resolution.
Through the combination of nanoscale Mie-resonance and photothermal/thermo-optical effect, plus a nanosecond excitation source that matches the thermal relaxation time of a silicon nanostructure, we demonstrated an ultra-large nonlinear index n2 = 1 um^2/mW, six-orders larger than the value in bulk. Under a confocal laser scanning scheme, unexpected sharp transition of scattering intensity is unveiled, suggesting a rapid temperature transient. The super-continuum wavelength tunability offers high-efficiency excitation among nano-silicon with various sizes. This robust and ultra-large nonlinearity shall be useful in optical switching and super-resolution mapping of semiconductor nanophotonic structures.
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