We present the ELAN testbed, which aims at assessing laser-induced damage of thick and large silica optics for the Laser Megajoule (LMJ) facility. A custom and patented injection seeding system was implemented on our Nd:YAG laser: this allows us to use phase modulated pulses to annihilate backward stimulated Brillouin scattering during tests while guaranteeing a smooth temporal profile. Then, beam propagation simulations of the incident spatial profile with Miro code (CEA) allows us to correct for the surface narrowing of the beam on the exit face of the optic due to Kerr self-focusing. This testbed allows us to test LMJ 34 mm vacuum window at 351 nm in nanosecond range with fluence up to 30-35 J/cm² with a control of non-linear propagation effect.
The paper aims to compare the results obtained with the same laser source with a large beam and with small beams. These latest were shaped from phase objects implemented to obtain several small beams from a single larger beam. The consistency of the results from both sets of measurements is shown. It validates the assumptions made and the specific mathematical treatments implemented to establish the link between the two approaches. It also validates and strengthens the approach developed from the rasterscan procedure used to measure damage densities from the scanning with beams of small dimensions. This shows that small beam tests are reasonably representative of tests carried out with large beams.
Laser damage resistance is a key factor for the operation and the improvement of high power laser systems. Up today laser damage performance of optical components is mainly a defect related material characteristic. Metrology procedures have been developed to realize repeatable and accurate measurements of surface damage density due to nanosecond pulses. These measurement techniques were used to guide the improvement of surface damage resistance. Fractures must be eliminated from surfaces, in order not to suffer a damage growth phenomenon, whose exponential character will reduce the optical lifetime. High intensity hot spots due to beam modulations, spatial and/or temporal modulations, can also cause surface damage. Specific set-ups and experiments were carried out that allowed us to analyze and explain these phenomena: damage initiation mechanisms, damage growth and beam propagation inside the optical components. The presentation aims to highlight relevant progress on these topics (1) initiation mechanisms due to defects show two phases: a first incubation phase followed by the expansion one of the damage site ; it appears also that damage diameters are well correlated with the expansion fluence, (2) a refined bulk observation coupled to a fractal analysis allow the quantification of bulk damage and therefore to explain the laser damage growth and its dependence on beam parameters like pulse length and fluence (3) non-linear amplification of phase and amplitude modulations lead to the amplification of the spatial pre-existing small scale modulations that increase the laser energy density locally and finally the number of damage sites. The whole of results, damage initiation, damage growth and beam propagation, is discussed to the light of the laser damage observed on LMJ optics.
A millimetric aperture Nd:glass laser system has been designed and constructed at the CEA-CESTA. Its aim is to best mimic the laser conditions that can be found in inertial confinement fusion facilities. It is therefore used to study the main phenomena that prevents these lasers to work at their maximum power: the laser induced damage of the optical components. The combination of temporal and spatial modulators provides, every minute, a 6 J, 7 mm, 351 nm homogeneous beam at the fused silica sample location. This proceeding illustrates the capacity of the facility over two experiments: the study of damage initiation and the growth of laser damage sites on fused silica, up to millimetric scales
The growth of damage sites from micrometric to millimetric scales under high energy laser system conditions
have herein been investigated. In this realm, a saturation of the surface growth followed by the rapid expansion of
radial cracks has been observed. This observation contrasts with the previously reported exponential behavior1
(for pulse durations above 2 ns) and linear behavior (for pulse durations below 2 ns). The observation of the
longitudinal damage structure coupled with fractal analysis has shown that these shifts in growth behavior seem
to be correlated with changes in the damage morphology.
The original damage ring pattern at the exit surface of fused silica induced by highly modulated nanosecond infrared laser pulses demonstrates the time dependence of damage morphology. Such a damage structure is used to study the dynamics of the plasma issued from open cracks. This pattern originates from electron avalanche in this plasma, which simultaneously leads to an ionization front displacement in air and a silica ablation process. Experiments have shown that the propagation speed of the detonation wave reaches about 20 km/s and scales as the cube root of the laser intensity, in good agreement with theoretical hydrodynamics modeling. During this presentation, we present the different phases and the associated mechanisms leading to this peculiar morphology: • During an incubation phase, a precursor defect provides energy deposit that drives the near surface material into a plasma state. • Next the silica plasma provides free electrons in the surrounding air, under laser irradiation an electron avalanche is initiated and generates a breakdown wave. • Then this breakdown wave leads to an expansion of the air plasma. This latter is able to heat strongly the silica surface as well as generate free electrons in its conduction band. Hence, the silica becomes activated along the breakdown wave. • When the silica has become absorbent, an ablation mechanism of silica occurs, simultaneously with the air plasma expansion, resulting in the formation of the ring patterns in the case of these modulated laser pulses. These mechanisms are supported by experiments realized in vacuum environment. A model describing the expansion of the heated area by thermal conduction due to plasma free electrons is then presented. Next, the paper deals with the two damage formation phases that are distinguished. The first phase corresponds to the incubation of the laser flux by a subsurface defect until the damage occurrence: an incubation fluence corresponds to this phase. The second is related to the damage expansion that only refers to the energy deposit feeding the activation mechanism up to the end of the pulse: an expansion fluence corresponds to this phase. A striking feature is that the damage diameters are proportional to the fluence of expansion at a given shot fluence. Indirectly, the fluences of incubation by the precursors are then determined.
Some silica plates of high power nanosecond lasers may be a few centimeter thick for instance because they should sustain vacuum. Measuring laser-induced damage thresholds at the output surface of these thick silica plates is a complex task because non-linear laser propagation effects may occur inside the plate which prevents knowing accurately the fluence at the output. Two non-linear effects have to be considered: stimulated Brillouin scattering (SBS) and Kerr effect. SBS is mainly driven by the spectral power density of the pulses: if the spectral power density is below a threshold, SBS is negligible. Thus, spectral broadening is required. Kerr effect depends on the instantaneous intensity. Hence, a smooth temporal shape without overshoots is required. However, both conditions (wide spectrum and no overshoots) are impossible to fulfill with standard lasers. As a matter of fact, an injected laser has a smooth temporal profile but is spectrally narrow. Without injection, the laser is multimode yielding a wide spectrum but a chaotic temporal profile. We solved the problem by phase-modulating a continuous-wave seeder of our laser (patent pending). The phasemodulation frequency is adjusted to a multiple of the inverse of the round-trip time of the laser cavity. The laser pulses have a wide spectrum to suppress SBS and do not exhibit temporal overshoots to reduce Kerr effects. During the presentation, we will show the features of the laser pulses and laser-induced damage measurements of thick silica plates using this scheme.
Seeded nanosecond Q-switched Nd:YAG lasers working with an unstable resonator and a variable-reflectivity-mirror are widely used for they represent useful sources for stable and repeatable light-matter-interaction experiments. Moreover, in most setups, the fundamental wavelength is converted to higher harmonics. When the injection seeder is turned off, random longitudinal mode beating occurs in the cavity, resulting in strong variations of the temporal profile of the pulses. The generated spikes can then be ten times higher than the maximum of equivalent seeded pulses. This strong temporal incoherence is shown to engender spatial incoherence in the focal plane of such unseeded pulses leading to an instantaneous angular displacement of tens of µrad. This effect is even more pronounced after frequency conversion.
The rasterscan procedure, developed to test large components, is an efficient method that allows measuring extremely low surface damage density (until 0.01 site/cm2 for large optics). This procedure was improved in terms of accuracy. The equipment, test procedure and data analysis to perform this damage test of large aperture optics are described. The originality of the refined procedure is that a shot to shot correlation is performed between the damage occurrence and the corresponding fluence by recording beam parameters of hundreds of thousands of shots during the qualification. Because tests are realized with small Gaussian beams (about 1mm @ 1/e), beam overlap and beam shape are key parameters which have to be taken into account in order to determine damage density. After complete data analysis and treatment, a repeatable metrology has been reached. The measurement is destructive for the sample. However the consideration of error bars on defects distributions allows us to compare data obtained on a same batch of optical components. This will permit to reach reproducible metrology. Then this procedure provides a straightforward means of comparing the experimental results obtained from several facilities using different lasers. Recently, an additional step has been added to the procedure, a growth step that permits considering only growing damage sites. To the end the lifetime of large optics on high power laser can be predicted.
With the purpose of understanding nanosecond laser induced damage mechanisms when working with multiple longitudinal mode pulses, an accurate measurement of the temporal profiles is required. In this study, the use of a streak camera with a wide bandwidth is justified through the knowledge of the Nd:YAG spectral characteristics. A statistical and phenomenological analysis of multiple longitudinal modes intensity profiles is then performed through experiments and modeling. The resolution limitation of our photodiodes is also discussed.
Laser damage growth on the exit surface of fused silica optics is considered as exponential, the growth coefficient depending essentially on fluence. In this presentation, experiments with large beams have been carried out at 351 nm under nanosecond pulses. A statistical analysis has then been conducted leading to a refined representation of the growth. The effect of several parameters has also been taken into account to describe precisely the growth phenomenon. Finally, the two main parameters reporting the growth are the mean fluence and the size of the damage sites. Contributions of other parameters have been estimated too: the number of neighbors around the damage site, the shot number.... From experimental results, a model based on a statistical approach has been developed that permits the description of a complete sequence of growth. At the end, the knowledge of damage initiation and damage growth permit the determination of the lifetime of optical components illuminated with successive shots.
The determination of surface damage densities of thick optical components is tricky due to the
occurrence of non-linear effects (Brillouin and Kerr) that affect the beam propagation through the
optics. It is then compulsory to record the beam parameters, mainly the temporal profile, in order to
predict and calculate fluence and/or intensity on the rear surface taking into account the non-linear
beam propagation.
Experiments have been realised with the use of large beams and several phase modulations were
activated, leading to numerous peak intensities due to the occurrence of temporal amplitude
modulations. Results are first compared in the case of thin optics in order to separate the intrinsic
absorptions by the defects which are the weak points of the optics to the effect of the non-linear
propagation. The correspondence between the length of the filaments and the beam parameters has been
realised in order to highlight the relevant beam parameters that have to be considered for the damage
test of thick optics. The whole of measurements and modeling permit us to measure more accurately the rear surface
damage of thick optics due to intrinsic defects.
KEYWORDS: Diagnostics, Near field, Optical amplifiers, Plasma, Mirrors, Frequency conversion, Calibration, Picosecond phenomena, Space operations, Fusion energy
The Laser Integration Line (LIL) was first designed as a prototype to validate the concepts and the laser architecture of
the Laser MegaJoule (LMJ). The LIL facility is a 4-beam laser representing a quad structure of the LMJ. A set of test
campaigns were conducted to safely ramp up laser performance. The main goal was to measure quad-specific features
such as beam synchronization and focal spot (size, smoothing contrast ratio or irradiation nonuniformity) versus the LMJ
requirements. Following the laser commissioning, the LIL has become a major instrument dedicated to the achievement
of plasma physics experiments for the French Simulation Program and was also opened to the academic scientific
community. One of the attributes of the LIL facility is to be very flexible to accommodate the requests of plasma
physicists during campaigns. The LIL is constantly evolving to best meet the needs of target physicists. Changes made or
planned are either to improve the quality of laser beams, or to increase the LIL Energy-Power operating space. To
optimize preparation and design of shot campaigns, the LIL performance status has been elaborated. It gives information
about the characteristics of the laser in terms of near field and far field, defines the steps to maintain performance,
explains how the facility responds to the request, details settings (smoothing, shaping of the focal spot, energy, temporal
pulse shaping, beam pointing) and gives the limits in energy and power. In this paper, an overview of the LIL
performance is presented.
The rasterscan test procedure implemented in order to determine low laser damage density of large aperture UV
fused silica optics was improved in terms of accuracy and repeatability. Tests have been carried on several facilities
using several pulse durations and spatial distributions. We describe the equipment, test procedure and data analysis to
perform this damage test with small beams (Gaussian beams, about 1mm @ 1/e, and top hat beams). Then, beam overlap
and beam shape are the two key parameters which are taken into account in order to determine damage density. After
data analysis and treatment, a repeatable metrology has been obtained. Moreover, the consideration of error bars on
defects distributions permits to compare data between these installations. This allows us to look for reproducibility, a
necessary condition in order to share results and to make reliable predictions of laser damage resistance. For that, a
careful attention has been paid to beam analysis.
KEYWORDS: Laser induced damage, Optical components, High power lasers, Fusion energy, Interferometry, Near field optics, Near field, Photodiodes, Image processing, Laser beam propagation
LIL and LMJ are two French high power lasers dedicated to fusion and plasma experiments. Mastering the
characteristics of the focal spots focused on the targets during the experiments is very important. In order to analyze the
focal spots in its high power lasers, the CEA has developed an independent set-up that enables to measure energy spatial
profiles over a 5 decade dynamic range by the means of several acquisitions taken at different power levels. The different
data sets are then stitched to obtain a high dynamic picture of the beam. The experiment can also be used as a photometer
enabling to measure the energy transmitted by an optical component. We used this set-up to study the effect of different
parameters on the energy spatial profile of the focal spots. We have measured the effect of laser damages (on the optical
components of the beam) on the energy scattered around the main focal spot. We also demonstrated that the level of this
scattered power can be calculated from a near-field picture of the beam or even with pictures of the damaged components
taken with an appropriate lighting.
A rasterscan test procedure [L. Lamaignère et al, Rev. Sci. Instrumen. 78, 103105 (2007)] has been
implemented in order to determine low laser damage density of large aperture UV fused silica optics. This
procedure was improved in terms of accuracy and repeatability. Tests have been carried on several facilities
using several pulse durations and spatial distributions. We describe the equipment, test procedure and data
analysis to perform this damage test with small beams (Gaussian beams, about 1mm @ 1/e, and top hat beams).
Then, beam overlap and beam shape are the two key parameters which are taken into account in order to
determine damage density. After data analysis and treatment, a repeatable metrology has been obtained.
Moreover, the consideration of error bars on defects distributions permits to compare data between these
installations. This allows us to reach reproducibility, a necessary condition in order to share results and to make
reliable predictions of laser damage resistance.
A rasterscan test procedure [L. Lamaignère et al, Rev. Sci. Instrumen. 78, 103105 (2007)] has been implemented
in order to determine low laser damage density of large aperture UV fused silica optics. This procedure was improved in
terms of accuracy and repeatability and is now used for the determination of bulk damage density for KDP crystals. The
large area (volume) scanned during tests permits to measure very low damage density. On small samples, small area are
tested using the normalized 1/1 test procedure consisting on the irradiation of few sites at several fluences. The classical
damage probability plot is converted in terms of damage density. The two testing procedures are complementary: the 1/1
mode is practical to test a wide fluence range while the rasterscan mode allows exploring low damage densities with
higher accuracy.
Tests have been carried out on several facilities using several pulse durations and spatial distributions. We
describe the equipment, test procedure and data analysis to perform this damage test with small beams (Gaussian beams,
about 1mm @ 1/e, and top hat beams). Then, beam overlap and beam shape are the two key parameters which are taken
into account in order to determine damage density. After data analysis and treatment, a repeatable metrology has been
obtained. Moreover, the consideration of error bars on defects distributions permits to compare data between these
installations. This allows us to reach reproducibility, a necessary condition in order to share results and to make reliable
predictions of laser damage resistance.
Other tests are realized with larger beams (centimeter sized) and with a single shot. Due to a large beam contrast,
a large fluence range is then covered. Then after data treatment, we find a good correlation between tests realised with
small and large beams. This allows us to make tests with different laser characteristics (spectral modulations, pulse
duration, laser polarisation) and then to study their influences on laser damage.
Significant improvement in polishing processes of fused silica optical components, has increased optics lifetime at the
wavelength of 351 nm. Nonetheless, for large laser operation facilities like the Laser MegaJoule (LMJ), zero defect
optics are not yet available. Therefore a damage mitigation technique has been developed to prevent the growth of
initiated damage sites: this technique consists in a local melting and evaporation of silica by CO2 laser irradiation on the
damage site. Because of the difficulty to produce efficient mitigated sites with large depth, the initial depth of damage to
mitigate is a critical issue. An aim of our work was to determine the real extension of the damage site (including
fractures) for different laser pulse durations between 3 ns and 16 ns and at different laser fluences. The fractures are nondetectable
in conventional microscopy. The depth of the damage can thus be underestimated. Hence confocal microscopy, was used to observe these sub-surface fractures and to measure precisely the depth of damage. Results show that the damage is 2 to 4 times wider than deeper and this ratio is independent of the pulse duration and of the fluence. With this new information, the mitigation process can now be optimized.
During the life of a high-power laser chain, optical components may be damaged due to local high fluence levels in the
inhomogeneous beam. The origin of the laser damage can be impurities, surface defects or flaws and cracks resulting
from polishing, or it may be produced by self-focusing in the component. The aim of this study is to better understand
the correlation between a surface crack on a silica optical component and laser damage. To accomplish this, calibrated
indentations were made on silica samples. Observations of the sites were made with an optical microscope, and three
different morphologies were recognized. Then the zones containing the indentations were irradiated (single shot mode)
with a Nd Yag laser at 355 nm for various fluences. Subsequent observations of the sites were made with an optical
microscope, with the aim of correlating site morphology and laser-induced damage. Some sites were believed to have
undergone laser conditioning. They were further irradiated (raster scan mode) at high fluence, and some evidence for a
laser conditioning effect was obtained.
A major issue in high power lasers for fusion is laser-induced damage on optical components. Since damage is often initiated by a surface crack resulting from polishing, it is important to understand the physics involved in this phenomenon. In this study, calibrated surface scratches have been realized on two silica samples using an indenter-scratcher apparatus. A variety of scratches have been tested by applying different speeds and forces on the scratcher needle. Optical microscope observations show that the scratches made at highest speed create irregular dashed lines. In addition, we have observed, at intermediate speed, an evolution in time of the scratches due to local stresses in silica.
One of the samples was irradiated by a Nd:YAG laser beam at 355 nm with the scratches on the exit surface. Microscope observations were made before and after irradiation.
Strong dependence on the scratch speed was observed on the local laser damage. Again, temporal evolution of the damage has been observed.
This paper presents data reduction on an experimental set-up that we have recently developed at CESTA, France. It has been implemented to analyze laser-induced damage on optics dedicated to the Megajoule laser project. Our goal is to measure the damage fluence on samples under tests, using a statistical approach on a very large number of sites.
The laser-induced damage density is accurately plotted as a function of laser fluence, by measuring the fluence of every single shot during the scan. This improvement of accuracy modifies dramatically the interpretation of the results that can be made, compared to raw data, considering the mean fluence only.
A major issue in high power lasers for fusion is laser-induced damage on optics and its evolution in time after a large number of shots. Since damage is often characterized by an initial surface crack, its surface usually increases, following an exponential law.
Surface scratches have been made on silica samples in order to get calibrated fractures. Then, to test different experimental conditions, we made a variety of scratches in terms of length and depth. The samples are then irradiated by a Nd:YAG laser first at 1064 nm (1w) then at 355 nm (3w). They are successively tested with the scratches facing the laser beam or placed with the scratches on the back surface.
To obtain better understanding of particulate contamination, chromium dots (50 x 50 μm2) were deposited on a silica substrate by photolithography. The aim in using this sample is to observe the mechanism of damage initiation that can be attributed to surface contamination of micro-metric size. A Nd:YAG laser irradiated the sample at 1064 nm for different fluences and also different numbers of shots. Several methods were used to characterise the laser effects on the chromium dots and the silica substrate: "Nomarski", "atomic force" and photothermal microscope observations.
The laser fluence is found to be the most important parameter for the behaviour of the chromium dots. At low fluence (<1 J/cm2), they become cracked (fractured). At medium fluence (around 1 J/cm2) chromium fusion is reached and chromium oxide appears. Finally at higher fluence (3 J/cm2), although chromium dots are blown off the substrate and small damage to silica occurs on the first shot, the subsequent shots do not lead to a dramatic increase in the damage.
Experiments have been performed to measure the rate of laser-induced damage growth at the rear surface of fused silica windows at 1064, 1053 and 351 nm. One test bench delivered 9 ns monomode gaussian pulses at 10 Hz and 1064 nm. The size of the focused beam on the sample was a few mm2. Another test bench delivered 2.5 ns single or multimode pulses at 1053 and 351 nm. The focused spot on the sample was a few cm2. We compare and discuss our laboratory experimental results, the larger scale ALISE laser data and other results obtained at LULI.
The functional lifetime of large aperture optical components used in high power lasers, like LIL and LMJ facilities, is mainly determined by laser damage measurements. We present experimental procedures and statistical analysis, made on small samples with mm-size beams, to determine damage densities and damage growth laws. The tests and analysis are compared to other results obtained with larger beams (few cm2) on large aperture components.
The functional lifetime of large aperture components used in high power lasers, like LIL and LMJ facilities, is mainly determined by laser damage measurements. Automatic damage test benches allow to obtain more data in less time than traditional tests. We present, first experimental procedures and statistical analysis made on small samples with mm-size beams, to determine damage densities and damage growth laws. The presented methods are the usual 1on1, Non1, Ron1 and Son1 tests and more specially the raster scan procedure. The tests and analysis are compared to other results obtained with larger beams (few cm2) on large optics. We show that the exact knowledge of each shot parameters (energy, surface and pulse duration) permits to determine the damage growth rate (and then to predict the lifetime of each optics), to precisely study self-focusing phenomenon and more to finely observe pre-damage-levels. In this way, the main parameters like fluence or intensity are associated to the observed phenomenon. Moreover laser beam diagnostics, many diagnostics used for the detection and the observation of damage occurrence are equally very important. It is also necessary to develop test procedures entirely computed which permit to scan all the surface of a component and to acquire in real time the beam parameters and the results of laser-matter interaction. Experimental results are reported to illustrate what could be achieved on an instrumented and automated facility.
The LMJ target chamber is designed to withstand high fusion energy produced by 20 MJ yield shots and 600 nm yield shots per year on a large variety of targets. We show how the target chamber and its equipment have to be protected from damaging by 14 MeV neutrons, high x-ray fluences, debris and shrapnel. A first wall made of louvers is required to prevent material ablated by x-rays form reaching the debris shields and reducing their live time. Constraints on the target design is also considered to limit the sources of vaporized or ionized mass and shrapnel coming directly from the target. The use of pre-shield for large mass targets is suggested to meet the requirement on the frequency cleaning of the debris shields.
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